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I don't understand what you are asking. Are you trying to paint the grill surround, or the grill itself? I'm not sure about what you are trying to paint..
Yeah you can paint it.. Like he said though ^^ you really gotta sand the **** outa chrome to get paint to stick. Will be easy for the grill surround but the billet grill might be difficult.
If your gonna paint any kind of metal you should try and sand it down as best as you can, regardless. Following that with primer would probably be a good idea too lol